Search results for "photo polymerization"

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Influence of a Crosslinker Containing an Azo Group on the Actuation Properties of a Photoactuating LCE System

2016

Photoactuating liquid crystalline elastomers (LCE) are promising candidates for an application as artificial muscles in microdevices. In this work, we demonstrate that by optimizing (1) the illumination conditions and (2) the mixture of azo monomer and azo crosslinker, thick films of an all-azo LCE can be prepared, which show a strong length change without bending during photoactuation. This becomes possible by working with white light (about 440 nm), whose absorption is low, leading to a large penetration depth. By adding an azo crosslinker to a previously prepared system, several improvements of the actuation properties—like a stronger photoactuation at lower operational temperatures—coul…

Materials sciencePolymers and Plasticsvis photo polymerizationazo02 engineering and technology010402 general chemistryElastomer01 natural sciencesArticleIsothermal processlcsh:QD241-441chemistry.chemical_compoundlcsh:Organic chemistryPolymer chemistryphotoactuationliquid crystalline elastomersIrradiationPenetration depthAbsorption (electromagnetic radiation)crosslinkerlight-responsiveactuatorpolymer filmGeneral Chemistry021001 nanoscience & nanotechnology0104 chemical sciencesliquid crystalline networkPhotopolymerMonomerChemical engineeringchemistryliquid crystalline elastomers; photoactuation; polymer film; light-responsive; azo; crosslinker; actuator; vis photo polymerization; liquid crystalline networkArtificial muscle0210 nano-technologyPolymers
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Microfluidic Synthesis of Actuating Microparticles from a Thiol-Ene Based Main-Chain Liquid Crystalline Elastomer.

2016

In this article the microfluidic synthesis of strongly actuating particles on the basis of a liquid crystalline main-chain elastomer is presented. The synthesis is carried out in a capillary-based co-flow microreactor by photo-initiated thiol-ene click chemistry of a liquid crystalline monomer mixture. These microparticles exhibit a deformation from a spherical to a rod-like shape during the thermal-initiated phase transition of the liquid crystalline elastomer (LCE) at which the particles’ aspect ratio is almost doubled. Repeated contraction cycles confirm the complete reversibility of the particles’ actuation properties. The transition temperature of the LCE, the temperature range of the …

Phase transitionMaterials sciencePolymers and PlasticsCapillary actionMicrofluidicsmicrofluidicsoft actuator02 engineering and technologycontinuous flow synthesis010402 general chemistryElastomer01 natural sciencesArticlestimuli-responsivelcsh:QD241-441Physics::Fluid Dynamicschemistry.chemical_compoundphoto polymerizationlcsh:Organic chemistryLiquid crystalliquid crystalComposite materialmicrofluidic; microparticles; liquid crystal; stimuli-responsive; soft actuator; thiol-ene; liquid crystalline elastomer; photo polymerization; continuous flow synthesismicroparticlesthiol-eneGeneral ChemistryAtmospheric temperature range021001 nanoscience & nanotechnology0104 chemical sciencesCondensed Matter::Soft Condensed MatterMonomerchemistryliquid crystalline elastomerMicroreactor0210 nano-technologyPolymers
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